Manipulation and characterization of xenon-metalloporphyrin complexation with a scanning tunneling microscope

J Am Chem Soc. 2002 Dec 11;124(49):14804-9. doi: 10.1021/ja0272639.

Abstract

The formation of a series of Xe-CuEtioI [Cu(II) etioporphyrin I] complexes on Cu(001) surface was identified by scanning tunneling microscopy (STM) at cryogenic condition. The binding sites of xenon to CuEtioI molecule were directly revealed by high-resolution STM images in combination with controlled manipulation. The interaction between xenon atoms and CuEtioI in the on-top configuration is suggestive of a charge-induced dipole interaction. The structural parameters obtained with the STM complement results from spectroscopic studies of van der Waals complexes.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Copper / chemistry
  • Metalloporphyrins / chemistry*
  • Microscopy, Scanning Tunneling
  • Surface Properties
  • Xenon / chemistry*

Substances

  • Metalloporphyrins
  • Xenon
  • Copper