A total synthesis prompts the structure revision of haouamine B

J Am Chem Soc. 2012 Jun 6;134(22):9291-5. doi: 10.1021/ja301326k. Epub 2012 May 23.

Abstract

A concise asymmetric approach to the indeno-tetrahydropyridine core of the unusual alkaloid haouamine B allowed for an investigation of a biomimetic oxidative phenol coupling as a proposed biosynthetic step, and ultimately provided access to the published structure of the natural product. As a consequence of our synthetic studies, the structure of haouamine B has been revised.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Heterocyclic Compounds, 4 or More Rings / chemical synthesis*
  • Heterocyclic Compounds, 4 or More Rings / chemistry
  • Molecular Structure

Substances

  • Heterocyclic Compounds, 4 or More Rings
  • haouamine B