Mapping Plant Phosphoproteome with Improved Tandem MOAC and Label-Free Quantification

Methods Mol Biol. 2021:2358:105-112. doi: 10.1007/978-1-0716-1625-3_7.

Abstract

Protein phosphorylation represents a fundamental and evolutionarily conserved type of posttranslational modification that regulates protein functions and cellular signal transmission. Due to the dynamic nature of protein phosphorylation processes in plant cells, large-scale studies of phosphoproteins face several challenges such as low stoichiometry in the modified peptides in a proteome, as well as heterogeneity of the phosphopeptides of a given protein. Here we describe an updated tandem MOAC combined phosphoprotein and phosphopeptide enrichment strategy, a scalable phosphoproteomics approach that allows identification of thousands of phophopeptides in plant materials in one LC-MS analysis. We implemented modifications to several steps of the original tandem MOAC procedure to increase the identification and quantification of phosphopeptides in a sample beginning with less amount of tissue and a smaller amount of extracted protein.

Keywords: Metabolism; Phosphorylation; Proteomics; Tandem MOAC.

MeSH terms

  • Chromatography, Liquid
  • Phosphopeptides / metabolism
  • Phosphoproteins / metabolism
  • Phosphorylation
  • Proteome* / metabolism
  • Proteomics
  • Tandem Mass Spectrometry

Substances

  • Phosphopeptides
  • Phosphoproteins
  • Proteome