Scalable and Tunable In-Plane Ge/Si(001) Nanowires Grown by Molecular Beam Epitaxy

Nano Lett. 2025 Jun 26. doi: 10.1021/acs.nanolett.5c02477. Online ahead of print.

Abstract

Germanium nanostructures offer significant potential in developing advanced integrated circuits and disruptive quantum technologies, yet achieving both scalability and high carrier mobility remains a challenge in materials science. Here, we report an original low-temperature epitaxial method for the growth of site-controlled in-plane germanium nanowires with high hole mobility by molecular beam epitaxy. By reducing the growth temperature, we effectively suppress Si-Ge interdiffusion, ensuring pure germanium composition within the nanowires while preserving their high crystalline quality. The method employs prepatterned ridges on strain-relaxed Si0.75Ge0.25/Si(001) substrates as tailored templates, enabling control over the position, length, spacing, and cross-sectional shape of the nanowires. Electrical measurements of field-effect devices made from as-grown germanium nanowires show that the nanowires are of hole conduction with mobility exceeding 7000 cm2/(V s) at 2-20 K. The method paves a way for fabrication of scalable germanium nanowire networks, providing a reliable platform for the developments of high-performance nanoelectronics and multiqubit chips.

Keywords: Germanium Nanowire; Hole Mobility; Molecular Beam Epitaxy; Quantum Technology; Site-Controlled Growth; Strain-Relaxed Substrate.